2019Physical review. B./Physical review. BOpen access

Non-Kitaev spin liquids in Kitaev materials

Yaodong Li, Yang Xu, Yi Zhou, Gang Chen

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Abstract

We point out that the Kitaev materials may not necessarily support Kitaev spin liquid. It is well known that having a Kitaev term in the spin interaction is not the sufficient condition for the Kitaev spin-liquid ground state. Many other spin liquids may be stabilized by the competing spin interactions of the systems. We thus explore the possibilities of non-Kitaev spin liquids in the honeycomb Kitaev materials. We carry out a systematic classification of gapped ${\mathbb{Z}}_{2}$ spin liquids using the Schwinger boson representation for the spin variables. The presence of strong spin-orbit coupling in the Kitaev materials brings new ingredients into the projective symmetry group classification of the non-Kitaev spin liquid. We predict the spectroscopic properties of these gapped non-Kitaev spin liquids. Moreover, among the gapped spin liquids that we discover, we identify the spin liquid whose spinon condensation leads to the zigzag magnetic order that was observed in ${\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}$ and $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$. We further discuss the possibility of gapped ${\mathbb{Z}}_{2}$ spin liquid and the deconfined quantum criticality from the zigzag magnetic order to spin dimerization in pressurized $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$.

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We point out that the Kitaev materials may not necessarily support Kitaev spin liquid. It is well known that having a Kitaev term in the spin interaction is not the sufficient condition for the Kitaev spin-liquid ground state. Many other spin liquids may be stabilized by the competing spin interactions of the systems. We thus explore the possibilities of non-Kitaev spin liquids in the honeycomb Kitaev materials. We carry out a systematic classification of gapped ${\mathbb{Z}}_{2}$ spin liquids using the Schwinger boson representation for the spin variables. The presence of strong spin-orbit coupling in the Kitaev materials brings new ingredients into the projective symmetry group classification of the non-Kitaev spin liquid. We predict the spectroscopic properties of these gapped non-Kitaev spin liquids. Moreover, among the gapped spin liquids that we discover, we identify the spin liquid whose spinon condensation leads to the zigzag magnetic order that was observed in ${\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}$ and $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$. We further discuss the possibility of gapped ${\mathbb{Z}}_{2}$ spin liquid and the deconfined quantum criticality from the zigzag magnetic order to spin dimerization in pressurized $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$.

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Available abstract

We point out that the Kitaev materials may not necessarily support Kitaev spin liquid. It is well known that having a Kitaev term in the spin interaction is not the sufficient condition for the Kitaev spin-liquid ground state. Many other spin liquids may be stabilized by the competing spin interactions of the systems. We thus explore the possibilities of non-Kitaev spin liquids in the honeycomb Kitaev materials. We carry out a systematic classification of gapped ${\mathbb{Z}}_{2}$ spin liquids using the Schwinger boson representation for the spin variables. The presence of strong spin-orbit coupling in the Kitaev materials brings new ingredients into the projective symmetry group classification of the non-Kitaev spin liquid. We predict the spectroscopic properties of these gapped non-Kitaev spin liquids. Moreover, among the gapped spin liquids that we discover, we identify the spin liquid whose spinon condensation leads to the zigzag magnetic order that was observed in ${\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}$ and $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$. We further discuss the possibility of gapped ${\mathbb{Z}}_{2}$ spin liquid and the deconfined quantum criticality from the zigzag magnetic order to spin dimerization in pressurized $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$.

Key concepts: Spinon, Quantum spin liquid, Spin (aerodynamics), Physics, Zigzag, Condensed matter physics, Order (exchange), Quantum mechanics

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