2008•ChemPhysChemRequires access

Resonance Raman Cross‐Sections and Vibronic Analysis of Rhodamine 6G from Broadband Stimulated Raman Spectroscopy

Sangdeok Shim, Christina M. Stuart, Richard A. Mathies

Abstract

Molecular resonance quantified: The resonance Raman spectrum of rhodamine 6G is obtained at 532 nm and the scattering cross-sections are quantified using resonance broadband stimulated Raman spectroscopy. Thus, the molecular resonance and surface-enhanced effects in SERRS are quantified for the first time. The surface enhancement is ∼107–108 in typical SERRS experiments.

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Key concepts: Raman spectroscopy, Rhodamine 6G, Resonance Raman spectroscopy, Resonance (particle physics), Raman scattering, Coherent anti-Stokes Raman spectroscopy, Chemistry, Spectroscopy