2010•Chemistry - A European JournalRequires access

Influence of the N‐Bridging Ligand on Magnetic Relaxation in an Organometallic Dysprosium Single‐Molecule Magnet

Richard A. Layfield, Joseph J. W. McDouall, Scott A. Sulway, Floriana Tuna, David J. Collison, Richard E. P. Winpenny

Abstract

Organometallic single-molecule magnet: Studies of two dimeric organometallic dysprosium compounds reveal one to be the first organometallic single-molecule magnet (see picture). A comparison of the magnetic properties and electronic structures of the two compounds shows that Dy⋅⋅⋅Dy interactions have a profound influence on the dynamic magnetic behaviour, while having little effect on the static magnetic measurements.

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Key concepts: Dysprosium, Single-molecule magnet, Magnet, Group 2 organometallic chemistry, Molecule, Crystallography, Magnetic relaxation, Lanthanide