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Doppler-Free Laser Polarization Spectroscopy

Carl Wieman, Theodor W. Hänsch

Open publisher page 773 citations

Abstract

We have demonstrated a sensitive new method of Doppler-free spectroscopy, monitoring the nonlinear interaction of two monochromatic laser beams in an absorbing gas via changes in light polarization. The signal-to-background ratio can greatly surpass that of saturated absorption. Polarization spectra of the hydrogen Balmer-$\ensuremath{\beta}$ line, recorded with a cw dye laser, reveal the Stark splitting of single fine-structure components in a Wood discharge.

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What this paper is about

We have demonstrated a sensitive new method of Doppler-free spectroscopy, monitoring the nonlinear interaction of two monochromatic laser beams in an absorbing gas via changes in light polarization. The signal-to-background ratio can greatly surpass that of saturated absorption. Polarization spectra of the hydrogen Balmer-$\ensuremath{\beta}$ line, recorded with a cw dye laser, reveal the Stark splitting of single fine-structure components in a Wood discharge.

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Available abstract

We have demonstrated a sensitive new method of Doppler-free spectroscopy, monitoring the nonlinear interaction of two monochromatic laser beams in an absorbing gas via changes in light polarization. The signal-to-background ratio can greatly surpass that of saturated absorption. Polarization spectra of the hydrogen Balmer-$\ensuremath{\beta}$ line, recorded with a cw dye laser, reveal the Stark splitting of single fine-structure components in a Wood discharge.

Key concepts: Balmer series, Monochromatic color, Polarization (electrochemistry), Spectroscopy, Absorption spectroscopy, Laser, Doppler effect, Materials science

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