2011•Radiochimica ActaRequires access

Investigation of the 236U/238U isotope abundance ratio in uranium ores and yellow cake samples

Michaela Srncik, Klaus Mayer, Erich Hrnecek, Maria Wallenius, Zsolt Varga, Peter Steier, Gabriele Wallner

Open publisher page 30 citations

Abstract

Abstract Uranium ores and yellow cake samples of known geographic origin were investigated for their n(236U)/n(238U) isotope abundance ratio. Samples from four different uranium mines in Australia, Brazil and Canada were selected. Uranium was separated by UTEVA® Resin and was measured by Accelerator Mass Spectrometry (AMS) at the Vienna Environmental Research Accelerator (VERA). The measurement of the isotope abundance ratio n(236U)/n(238U) will be used to investigate possible correlations between the original mineral (uranium ore) and the intermediate product (yellow cake). Such correlations are useful indicators for nuclear forensic or for non-proliferation purposes.

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Abstract Uranium ores and yellow cake samples of known geographic origin were investigated for their n(236U)/n(238U) isotope abundance ratio. Samples from four different uranium mines in Australia, Brazil and Canada were selected. Uranium was separated by UTEVA® Resin and was measured by Accelerator Mass Spectrometry (AMS) at the Vienna Environmental Research Accelerator (VERA). The measurement of the isotope abundance ratio n(236U)/n(238U) will be used to investigate possible correlations between the original mineral (uranium ore) and the intermediate product (yellow cake). Such correlations are useful indicators for nuclear forensic or for non-proliferation purposes.

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Available abstract

Abstract Uranium ores and yellow cake samples of known geographic origin were investigated for their n(236U)/n(238U) isotope abundance ratio. Samples from four different uranium mines in Australia, Brazil and Canada were selected. Uranium was separated by UTEVA® Resin and was measured by Accelerator Mass Spectrometry (AMS) at the Vienna Environmental Research Accelerator (VERA). The measurement of the isotope abundance ratio n(236U)/n(238U) will be used to investigate possible correlations between the original mineral (uranium ore) and the intermediate product (yellow cake). Such correlations are useful indicators for nuclear forensic or for non-proliferation purposes.

Key concepts: Uranium, Natural abundance, Isotope, Chemistry, Isotopes of uranium, Abundance (ecology), Radiochemistry, Isotopic ratio

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