2007Physical Review BOpen access

Superexchange induced canted ferromagnetism in dilute magnets

G. Bouzerar, R. Bouzerar, O. Cépas

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Abstract

We argue, in contrast to recent studies, that the antiferromagnetic superexchange coupling between nearest neighbor spins does not fully destroy the ferromagnetism in dilute magnets with long-ranged ferromagnetic couplings. Above a critical coupling, we find a canted ferromagnetic phase with unsaturated moment. We have calculated the transition temperature using a simplified local random phase approximation procedure which accounts for the canting. For dilute magnetic semiconductors, such as GaMnAs, using ab initio couplings allows us to predict the existence of a canted phase and provides an explanation for the apparent contradictions observed in experimental measurements. Finally, we compared with previous studies that used Ruderman-Kittel-Kasuya-Yosida couplings and reported nonferromagnetic states when the superexchange is too strong. Even in this case the ferromagnetism should remain essentially stable in the form of a canted phase.

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We argue, in contrast to recent studies, that the antiferromagnetic superexchange coupling between nearest neighbor spins does not fully destroy the ferromagnetism in dilute magnets with long-ranged ferromagnetic couplings. Above a critical coupling, we find a canted ferromagnetic phase with unsaturated moment. We have calculated the transition temperature using a simplified local random phase approximation procedure which accounts for the canting. For dilute magnetic semiconductors, such as GaMnAs, using ab initio couplings allows us to predict the existence of a canted phase and provides an explanation for the apparent contradictions observed in experimental measurements. Finally, we compared with previous studies that used Ruderman-Kittel-Kasuya-Yosida couplings and reported nonferromagnetic states when the superexchange is too strong. Even in this case the ferromagnetism should remain essentially stable in the form of a canted phase.

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Available abstract

We argue, in contrast to recent studies, that the antiferromagnetic superexchange coupling between nearest neighbor spins does not fully destroy the ferromagnetism in dilute magnets with long-ranged ferromagnetic couplings. Above a critical coupling, we find a canted ferromagnetic phase with unsaturated moment. We have calculated the transition temperature using a simplified local random phase approximation procedure which accounts for the canting. For dilute magnetic semiconductors, such as GaMnAs, using ab initio couplings allows us to predict the existence of a canted phase and provides an explanation for the apparent contradictions observed in experimental measurements. Finally, we compared with previous studies that used Ruderman-Kittel-Kasuya-Yosida couplings and reported nonferromagnetic states when the superexchange is too strong. Even in this case the ferromagnetism should remain essentially stable in the form of a canted phase.

Key concepts: Superexchange, Condensed matter physics, Ferromagnetism, Antiferromagnetism, Spins, Coupling (piping), Phase (matter), Phase transition

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