2011•Physical Review BOpen access

Extended Drude model and role of interband transitions in the midinfrared spectra of pnictides

Lara Benfatto, E. Cappelluti, Luciano Ortenzi, Lilia Boeri

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Abstract

We analyze the outcomes of an extended-Drude-model approach to the optical spectra of pnictides, where the multiband nature of the electronic excitations requires a careful analysis of the role of interband processes in the optical conductivity. Through a direct comparison between model calculations of the intraband optical spectra, experimental data, and first-principles calculations we show that interband transitions give a non-negligible contribution already in the infrared region. This leads to a substantial failure of the extended-Drude-model analysis on the measured optical data without subtraction of interband contributions.

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We analyze the outcomes of an extended-Drude-model approach to the optical spectra of pnictides, where the multiband nature of the electronic excitations requires a careful analysis of the role of interband processes in the optical conductivity. Through a direct comparison between model calculations of the intraband optical spectra, experimental data, and first-principles calculations we show that interband transitions give a non-negligible contribution already in the infrared region. This leads to a substantial failure of the extended-Drude-model analysis on the measured optical data without subtraction of interband contributions.

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Available abstract

We analyze the outcomes of an extended-Drude-model approach to the optical spectra of pnictides, where the multiband nature of the electronic excitations requires a careful analysis of the role of interband processes in the optical conductivity. Through a direct comparison between model calculations of the intraband optical spectra, experimental data, and first-principles calculations we show that interband transitions give a non-negligible contribution already in the infrared region. This leads to a substantial failure of the extended-Drude-model analysis on the measured optical data without subtraction of interband contributions.

Key concepts: Drude model, Optical conductivity, Spectral line, Optical spectra, Infrared, Condensed matter physics, Physics, Conductivity

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