2010Physical Review BRequires access

Self-diffusion in liquid copper as seen by quasielastic neutron scattering

Andreas Meyer

Open publisher page 106 citations

Abstract

Quasielastic neutron scattering has been used to study atomic dynamics in liquid Cu. At small wave numbers $q$ the intermediate scattering function is dominated by incoherent scattering contributions. From the decay of the quasielastic signal, self-diffusion coefficients $D$ are obtained on an absolute scale. In a temperature range from 1370 to 1620 K, $D$ values exhibit an Arrhenius-type temperature dependence and are significantly smaller than those from previous tracer experiments that are hampered by convective flow.

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What this paper is about

Quasielastic neutron scattering has been used to study atomic dynamics in liquid Cu. At small wave numbers $q$ the intermediate scattering function is dominated by incoherent scattering contributions. From the decay of the quasielastic signal, self-diffusion coefficients $D$ are obtained on an absolute scale. In a temperature range from 1370 to 1620 K, $D$ values exhibit an Arrhenius-type temperature dependence and are significantly smaller than those from previous tracer experiments that are hampered by convective flow.

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Available abstract

Quasielastic neutron scattering has been used to study atomic dynamics in liquid Cu. At small wave numbers $q$ the intermediate scattering function is dominated by incoherent scattering contributions. From the decay of the quasielastic signal, self-diffusion coefficients $D$ are obtained on an absolute scale. In a temperature range from 1370 to 1620 K, $D$ values exhibit an Arrhenius-type temperature dependence and are significantly smaller than those from previous tracer experiments that are hampered by convective flow.

Key concepts: Quasielastic neutron scattering, Quasielastic scattering, Arrhenius equation, Diffusion, Neutron scattering, Scattering, Materials science, Small-angle neutron scattering

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