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2009•Dalton TransactionsOpen access

Hydroamination reactions by metal triflates: Brønsted acid vs. metal catalysis?

Jason G. Taylor, Luis A. Adrio, King Kuok Hii

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Abstract

Catalytic hydroamination reactions involving the addition of carboxamides (X = CO), carbamates (X = CO(2)) and sulfonamides (X = SO(2)) to unactivated C=C bonds are briefly reviewed. Development in this field of catalytic research is briefly charted, followed by a discussion of possible mechanisms, including arguments to support the operation of both metal and Brønsted acid catalysis in these systems. Future developments in the area are summarised.

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What this paper is about

Catalytic hydroamination reactions involving the addition of carboxamides (X = CO), carbamates (X = CO(2)) and sulfonamides (X = SO(2)) to unactivated C=C bonds are briefly reviewed. Development in this field of catalytic research is briefly charted, followed by a discussion of possible mechanisms, including arguments to support the operation of both metal and Brønsted acid catalysis in these systems. Future developments in the area are summarised.

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Available abstract

Catalytic hydroamination reactions involving the addition of carboxamides (X = CO), carbamates (X = CO(2)) and sulfonamides (X = SO(2)) to unactivated C=C bonds are briefly reviewed. Development in this field of catalytic research is briefly charted, followed by a discussion of possible mechanisms, including arguments to support the operation of both metal and Brønsted acid catalysis in these systems. Future developments in the area are summarised.

Key concepts: Hydroamination, Catalysis, Brønsted–Lowry acid–base theory, Metal, Chemistry, Combinatorial chemistry, Organic chemistry

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