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Energy and angular differential probabilities for photoionization of He using chirped attosecond soft-x-ray pulses

Teck-Ghee Lee, Michael Stuart Pindzola, F. Robicheaux

Open publisher page 16 citations

Abstract

Based on the time-dependent close-coupling method, energy and angular differential probabilities for various ionization processes of He atoms subjected to intense attosecond soft-x-ray pulses with a photon energy of 91.6 eV and a peak intensity of ${10}^{15}\text{ }\text{W}/{\text{cm}}^{2}$ are calculated to explore their dependence on the duration and the chirp of the pulse. It is found that the single and the double electron energy distributions for two-photon double ionization are rather sensitive to chirps. That is, both the magnitudes and locations of the sequential peaks in the single electron energy distributions vary strongly with chirps and the two-electron energy distributions being broadened and stretched along the equal energy sharing direction as opposed to the usual total excess energy direction for the case of zero chirp. In addition, our calculation also reveals an unexpected structure formed between the two sequential peaks. In order to better understand the chirp effects on both independent-electron and correlated electron emissions and their relations to the origin of the structure, we analyzed the corresponding probability differential in energy and angle.

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Based on the time-dependent close-coupling method, energy and angular differential probabilities for various ionization processes of He atoms subjected to intense attosecond soft-x-ray pulses with a photon energy of 91.6 eV and a peak intensity of ${10}^{15}\text{ }\text{W}/{\text{cm}}^{2}$ are calculated to explore their dependence on the duration and the chirp of the pulse. It is found that the single and the double electron energy distributions for two-photon double ionization are rather sensitive to chirps. That is, both the magnitudes and locations of the sequential peaks in the single electron energy distributions vary strongly with chirps and the two-electron energy distributions being broadened and stretched along the equal energy sharing direction as opposed to the usual total excess energy direction for the case of zero chirp. In addition, our calculation also reveals an unexpected structure formed between the two sequential peaks. In order to better understand the chirp effects on both independent-electron and correlated electron emissions and their relations to the origin of the structure, we analyzed the corresponding probability differential in energy and angle.

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Available abstract

Based on the time-dependent close-coupling method, energy and angular differential probabilities for various ionization processes of He atoms subjected to intense attosecond soft-x-ray pulses with a photon energy of 91.6 eV and a peak intensity of ${10}^{15}\text{ }\text{W}/{\text{cm}}^{2}$ are calculated to explore their dependence on the duration and the chirp of the pulse. It is found that the single and the double electron energy distributions for two-photon double ionization are rather sensitive to chirps. That is, both the magnitudes and locations of the sequential peaks in the single electron energy distributions vary strongly with chirps and the two-electron energy distributions being broadened and stretched along the equal energy sharing direction as opposed to the usual total excess energy direction for the case of zero chirp. In addition, our calculation also reveals an unexpected structure formed between the two sequential peaks. In order to better understand the chirp effects on both independent-electron and correlated electron emissions and their relations to the origin of the structure, we analyzed the corresponding probability differential in energy and angle.

Key concepts: Physics, Attosecond, Photoionization, Atomic physics, Ionization, Chirp, Electron, Photon energy

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