Mass and Nuclear Charge Distributions from the Spontaneous Fission of Fm254
R.M. Harbour, K.W. MacMurdo, David E. Troutner, M. V. Hoehn
Abstract
R.M. Harbour, K.W. MacMurdo, David E. Troutner, M. V. Hoehn
Abstract
The relative fission yields of 20 mass chains from $^{254}\mathrm{Fm}$ spontaneous fission were measured by direct high-resolution $\ensuremath{\gamma}$-ray spectroscopy of the gross fission products. Reflected yields were calculated based on a prompt-neutron fission yield of 3.94; the absolute yields were determined by requiring the sum of all yields to be 200%. A peak-to-valley ratio for the mass-yield curve of \ensuremath{\ge}18 was determined radiochemically by measuring the cumulative yields of $^{140}\mathrm{Ba}$ and $^{127}\mathrm{Sb}$.$^{254}\mathrm{Fm}$ was produced by irradiating $^{253}\mathrm{Es}$ in a high-flux reactor and then chemically separating the 3.24-h $^{254}\mathrm{Fm}$ from its 39.3-h $^{254}\mathrm{Es}^{m}$ parent. An aluminum "catcher" foil was used to collect the $^{254}\mathrm{Fm}$ fission products. Nuclear charge distribution studies included measurements of the independent yields of $^{140}\mathrm{La}$, $^{135}\mathrm{Xe}$, $^{134}\mathrm{I}$, and $^{132}\mathrm{I}$ relative to their cumulative yields from direct $\ensuremath{\gamma}$-ray-spectroscopy data.
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The relative fission yields of 20 mass chains from $^{254}\mathrm{Fm}$ spontaneous fission were measured by direct high-resolution $\ensuremath{\gamma}$-ray spectroscopy of the gross fission products. Reflected yields were calculated based on a prompt-neutron fission yield of 3.94; the absolute yields were determined by requiring the sum of all yields to be 200%. A peak-to-valley ratio for the mass-yield curve of \ensuremath{\ge}18 was determined radiochemically by measuring the cumulative yields of $^{140}\mathrm{Ba}$ and $^{127}\mathrm{Sb}$.$^{254}\mathrm{Fm}$ was produced by irradiating $^{253}\mathrm{Es}$ in a high-flux reactor and then chemically separating the 3.24-h $^{254}\mathrm{Fm}$ from its 39.3-h $^{254}\mathrm{Es}^{m}$ parent. An aluminum "catcher" foil was used to collect the $^{254}\mathrm{Fm}$ fission products. Nuclear charge distribution studies included measurements of the independent yields of $^{140}\mathrm{La}$, $^{135}\mathrm{Xe}$, $^{134}\mathrm{I}$, and $^{132}\mathrm{I}$ relative to their cumulative yields from direct $\ensuremath{\gamma}$-ray-spectroscopy data.
Key concepts: Fission, Fission product yield, Physics, Charge (physics), Fission products, Yield (engineering), Gamma spectroscopy, Nuclear fission product