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Volatilization and reaction of fission products in flowing steam. [PWR; BWR]

Irving Johnson, David V. Steidl, C. E. Johnson

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Abstract

The principal risk to the public from nuclear power plants derives from the highly radioactive atoms (fission products) generated as energy is produced in the nuclear fuel. The revolatilization of fission products from reactor system surfaces due to self-heating by radioactive decay has become a complicating factor in the source-term redefinition effort. It has had a major impact on calculations of fission product distributions in accident safety analyses. The focus of this research effort was to investigate the volatilization and transport of fission products and control rod materials in a flowing gaseous steam-hydrogen mixture. Fission product and control rod materials in various combinations were studied including CsI, CsOH, TeO/sub 2/, SrO, Ag, In, Cd and Mn. The vaporization behavior of the deposits were characterized with respect to vaporization rates, chemical species and downstream transport behavior.

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What this paper is about

The principal risk to the public from nuclear power plants derives from the highly radioactive atoms (fission products) generated as energy is produced in the nuclear fuel. The revolatilization of fission products from reactor system surfaces due to self-heating by radioactive decay has become a complicating factor in the source-term redefinition effort. It has had a major impact on calculations of fission product distributions in accident safety analyses. The focus of this research effort was to investigate the volatilization and transport of fission products and control rod materials in a flowing gaseous steam-hydrogen mixture. Fission product and control rod materials in various combinations were studied including CsI, CsOH, TeO/sub 2/, SrO, Ag, In, Cd and Mn. The vaporization behavior of the deposits were characterized with respect to vaporization rates, chemical species and downstream transport behavior.

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Available abstract

The principal risk to the public from nuclear power plants derives from the highly radioactive atoms (fission products) generated as energy is produced in the nuclear fuel. The revolatilization of fission products from reactor system surfaces due to self-heating by radioactive decay has become a complicating factor in the source-term redefinition effort. It has had a major impact on calculations of fission product distributions in accident safety analyses. The focus of this research effort was to investigate the volatilization and transport of fission products and control rod materials in a flowing gaseous steam-hydrogen mixture. Fission product and control rod materials in various combinations were studied including CsI, CsOH, TeO/sub 2/, SrO, Ag, In, Cd and Mn. The vaporization behavior of the deposits were characterized with respect to vaporization rates, chemical species and downstream transport behavior.

Key concepts: Nuclear fission product, Fission products, Long-lived fission product, Vaporization, Nuclear engineering, Fuel element failure, Volatilisation, Radioactive waste

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