PRODUCTION OF SHORT LIVED RADIOACTIVE CESIUM
Naokazu Shibata, Hiroshi Amano, T. Kuroyanagi, Eiji Shikata, K. Tanaka, H. Ebihara, Tetsuya Tamura
Abstract
Naokazu Shibata, Hiroshi Amano, T. Kuroyanagi, Eiji Shikata, K. Tanaka, H. Ebihara, Tetsuya Tamura
Abstract
Production methods for short-lived Cs radioisotopes were studied by using the reactions: Cs/sup 133/( gamma ,n)Cs/sup 132/, Xe(p,xn)/sup */Cs; and Ba/ sup 130/(n, gamma yields EC)Cs/sup 131/. In the ( gamma ,n) reac tion, CsCl and CsNO/sub 3/ were bombarded with gamma rays converted from 20-Mev accelerated electrons. The target was carefully assembled in irradiation to make Cs/sup 132/ a high specific activity. The specific activity of the product in 10 hr irradiation was about 10 mC/g of Cs, and the yield was about 10 mC. The radiochemical purity was more taan 99.9%. Xe gas target, of more than 99% purity, was bombanded with 16-Mev protons accelerated by a 160-cm cyclotron. The radioactive Cs nuclides produced Cs/sup 129/, Cs/sup 132/, and others were collected on a negatively charged Pt wire and separated very simply from other by products. Cs/sup 131/ activity, which was produced by pile neutron irradiation and separated by the cation exchanger method, was 99% pure with an order of 10 mC. (P.C.H.)
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Production methods for short-lived Cs radioisotopes were studied by using the reactions: Cs/sup 133/( gamma ,n)Cs/sup 132/, Xe(p,xn)/sup */Cs; and Ba/ sup 130/(n, gamma yields EC)Cs/sup 131/. In the ( gamma ,n) reac tion, CsCl and CsNO/sub 3/ were bombarded with gamma rays converted from 20-Mev accelerated electrons. The target was carefully assembled in irradiation to make Cs/sup 132/ a high specific activity. The specific activity of the product in 10 hr irradiation was about 10 mC/g of Cs, and the yield was about 10 mC. The radiochemical purity was more taan 99.9%. Xe gas target, of more than 99% purity, was bombanded with 16-Mev protons accelerated by a 160-cm cyclotron. The radioactive Cs nuclides produced Cs/sup 129/, Cs/sup 132/, and others were collected on a negatively charged Pt wire and separated very simply from other by products. Cs/sup 131/ activity, which was produced by pile neutron irradiation and separated by the cation exchanger method, was 99% pure with an order of 10 mC. (P.C.H.)
Key concepts: Radiochemistry, Irradiation, Nuclide, Yield (engineering), Caesium, Chemistry, Nuclear reaction, Neutron