SPONTANEOUS-FISSION HALF-LIVES OF PLUTONIUM-240 AND PLUTONIUM-242
L.Z. Malkin, I. D. Alkhazov, A.S. Krivokhatskii, K.A. Petrzhak
Abstract
L.Z. Malkin, I. D. Alkhazov, A.S. Krivokhatskii, K.A. Petrzhak
Abstract
Previously published values of the half lives of Pu/sup 240/ and Pu/sup 242/ are not sufficiently accurate because only very small amounts of the isotopes were available. A series of measurements was started, using preparations with a small surface density and a high concentration of the isotope studied. A Xe-filled scintillation counter was used as the fission-fragment detector; its resolution was better than that of ionization chambers. Before starting the measurements, the counter was evacuated to 5 x 10/sup -7/ mm of Hg, then filled with Xe to a pressure of 2.5 to 3 atm. The stability of the system was tested by measuring the energy spectrum of U/sup 233/ fission fragments. The spontaneousfission half life of Pu was found to be (1.45 plus or minus 0.02) x 10/sup 11/ years, using a preparation with a surface density of 7 x l0 microgram/ cm and a Pu /sup 239//Pu/sup 240/ ratio of 7.04. A second series of tests with a preparation possessing a P /sup 240//P /sup 242/ == 1.24 ratio yielded a corresponding half life value of (7.45 plus or minus 0.17) x 10/sup 10/ years for Pu/sup 242/. The energy spectrum of the spontaneous fission fragments is alsomore » presented. (TTT)« less
OpenAlex reports 6 citations for this work. Citation counts describe recorded attention and do not establish research quality.
A contribution statement is not available in the OpenAlex record.
Method details are not available in the OpenAlex metadata.
Findings are not separately available in the OpenAlex metadata.
Limitations are not available in the OpenAlex metadata.
Application details are not available in the OpenAlex metadata.
Previously published values of the half lives of Pu/sup 240/ and Pu/sup 242/ are not sufficiently accurate because only very small amounts of the isotopes were available. A series of measurements was started, using preparations with a small surface density and a high concentration of the isotope studied. A Xe-filled scintillation counter was used as the fission-fragment detector; its resolution was better than that of ionization chambers. Before starting the measurements, the counter was evacuated to 5 x 10/sup -7/ mm of Hg, then filled with Xe to a pressure of 2.5 to 3 atm. The stability of the system was tested by measuring the energy spectrum of U/sup 233/ fission fragments. The spontaneousfission half life of Pu was found to be (1.45 plus or minus 0.02) x 10/sup 11/ years, using a preparation with a surface density of 7 x l0 microgram/ cm and a Pu /sup 239//Pu/sup 240/ ratio of 7.04. A second series of tests with a preparation possessing a P /sup 240//P /sup 242/ == 1.24 ratio yielded a corresponding half life value of (7.45 plus or minus 0.17) x 10/sup 10/ years for Pu/sup 242/. The energy spectrum of the spontaneous fission fragments is alsomore » presented. (TTT)« less
Key concepts: Fission, Plutonium, Spontaneous fission, Isotope, Plutonium-240, Plutonium-239, Radiochemistry, Analytical Chemistry (journal)